Given a consequence relation in many-valued logic, what connectives can be defined? For instance, does there always exist a conditional operator internalizing the consequence relation, and which form should it take? In this paper, we pose this question in a multi-premise multi-conclusion setting for the class of so-called intersective mixed consequence relations, which extends the class of Tarskian relations. Using computer-aided methods, we answer extensively for 3-valued and 4-valued logics, focusing not only on conditional operators, but also on what we (...) call Gentzen-regular connectives. For arbitrary N-valued logics, we state necessary and sufficient conditions for the existence of such connectives in a multi-premise multi-conclusion setting. The results show that mixed consequence relations admit all classical connectives, and among them pure consequence relations are those that admit no other Gentzen-regular connectives. Conditionals can also be found for a broader class of intersective mixed consequence relations, but with the exclusion of order-theoretic consequence relations. (shrink)